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A list containing the names of some one hundred and thirty-six former students of the Neuadd-lwyd school or academy ('Myfyrwyr Athrofa Neuaddlwyd'), giving in some instances, the dates of their entering the academy, of commencing their career in the ministry (where applicable), and of death. Occasionally, notes such as 'Went to America', or 'To Rotherham where he died', are added.

Deeds and documents, 1545-1831, relating mainly to the Rees family of Dyffryn Clettwr, Llanarth, Cardiganshire, (now NLW Deeds 433-473), and manuscripts relating to Neuaddlwyd and other Congregational chapels, 1791-1896, including letters from missionaries, 1821-1832 (now NLW MSS 19154-7).

Deeds, documents and business papers, 1843-1955, of the Evans family of Neuaddfawr and Rhydyronen, p. Llanfihangel Genau'r Glyn, Cardiganshire, together with poor rate books for the township of Trefeurig in the parish of Llanbadarn Fawr, [1850s]-[1860s] and an account book of Seion Independent Chapel in the township of Ceulan-a-Maesmor, 1857-1872.

Deeds, 1554-1915, relating to the Neuadd-fawr estates in Breconshire, Carmarthenshire, Cardiganshire and Radnorshire; together with some papers relating to the development of Llanwrtyd Wells, Breconshire, as a spa in the nineteenth century.

Manuscripts from the library of Sir Owen Morgan Edwards (1858-1920), mostly belonging to the nineteenth century, and consisting of original copy of published material in the form of essays, short stories, original and translated poetry, collections of proverbs, etc.; also included in the collection are account books, sermons, diary entries, miscellaneous papers on various literary topics, and autograph letters of well-known Welsh figures.

Llythyrau, 1914-1933, at Ellis D. Jones, yn bennaf yn ymwneud â sefydlu Neuadd Goffa Owain Glyndŵr yng Nglyndyfrdwy, 1931-1932, y gohebwyr yn cynnwys T. E. Ellis (3), T. Gwynn Jones (3) a Syr John Edward Lloyd (2), ynghŷd â llythyrau eraill, 1936-1952, rhai ohonynt wedi'u cyfeirio at Syr Alfred Thomas Davies a'r gohebwyr yn cynnwys Syr John Ballinger (1) a W. Ambrose Bebb (3); ac eitemau amrywiol sy'n cynnwys cynllun, 1932, ar gyfer plannu planhigion ar dir Neuadd Goffa Owain Glyndŵr, llyfr lloffion yn ymwneud yn bennaf â'r Neuadd Goffa, a nodiadau yn ymwneud ag Owain Glyndŵr, ac â threfn gwasanaeth sefydlu'r Neuadd Goffa, 5 Medi 1931 = Letters, 1914-1933, to Ellis D. Jones, mainly relating to the establishment of the Owain Glyndŵr Memorial Hall in Glyndyfrdwy, 1931-1932, the correspondents including T. E. Ellis (3), T. Gwynn Jones (3) and Sir John Edward Lloyd (2), together with other letters, 1936-1952, some of which are addressed to Sir Alfred Thomas Davies, the correspondents including Sir John Ballinger (1) and W. Ambrose Bebb (3); and miscellaneous items which include a proposed 'planting plan', 1932, for the Owain Glyndŵr Memorial Hall grounds, a scrap book mainly relating to the Memorial Hall, and notes relating to Owain Glyndŵr, and to the order of service at the establishment of the Memorial Hall, 5 September 1931.

A copy of Nesta L. Harries's study entitled 'The Welsh Woollen Industry' written for her final examination at St Catharine's College, Tottenham, London, early 1950s, and containing samples of materials produced in woollen mills throughout Wales.

Papers, 1618-1999, including letters and genealogical material relating to families connected with Nerquis Hall, Flintshire, together with rentals and accounts of the Halghton estate, 1722-1748, and rentals of the Gwernheulod estate, Flintshire, 1768, and the Pengwern estate, Merionethshire, 1806-1814. Additional deeds and papers relating to Pengwern Hall, 1919-1999, were received in 2006.

Papers, 1988-1995, accumulated by Neil Kinnock as MP for Islwyn, mainly comprising constituency correspondence, and papers relating to local affairs, including health and welfare, industry, local government and the closure of sub-post offices in South Wales.

Holograph, autograph, and typescript messages of greetings for publication in the first number of Y Cymro, 3 December, 1932. The writers include D[avid] Miall Edwards; Ifan ab Owen Edwards (with a covering letter from R. E. Griffith); D[avid] Emrys Evans, University College of North Wales, Bangor; D[avid] Tecwyn Evans; D[avid] Lloyd George (with a covering letter from A. J. Sylvester); Peter Hughes Griffiths; W. J. Gruffydd; E[dward] Ernest Hughes; John Jenkins ('Gwili'); C[adwaladr] Bryner Jones; and T. Gwynn Jones.

Records of the Nefyn Branch of the Caernarvon Conservative and Unionist Association, including a minute book, 1960-1979, and minute book of the womens' branch, 1960-1976; circulars, [1960s]-1977; miscellaneous papers, [1960s]-1979; and publications from the Conservative and Unionist Central Office, 1946-1977.

Papers from the collection of William Roberts which include correspondence; sermons; miscellaneous notes and accounts; volume four of an essay in five volumes on the poets and writers of Gwent and Glamorgan; and reports and accounts relating to collieries and iron-works in South Wales.

Rent roll, dated 8 November 1540 (32 Hen. VIII), of the manor of Neath Ultra, Glamorgan, in the court of Francise Sowthewell and William Pooke, commissioners for the king, arranged into free and customary tenants.

Rent roll, 1666, of the manor of Neath Ultra and Cilybebyll, Glamorgan, arranged into free, customary and demense tenants. Also a memorandum of the heriot due on the death, alienation, 'incomb or releife' of a free tenant and the death of a customary tenant.

Accounts, 1786-1800, of the overseers of the poor in the hamlet of Neath Lower, Glamorgan.

Near-final autograph draft of The Village The City The Village (1956) by Glyn Jones. (Formerly Glyn Jones MS 7.) English. Unbound. Purchased from Glyn Jones, 1971.

Papers relating to the navigation and the lighting of the river Dee, 1910.