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1952 and 1966: Llwyn estate records, mainly title deeds and abstracts of title, 1623-1932, together with a few business letters, plans, printed sale catalogues and rentals, 1855-1908, relating to properties principally in Llanfyllin (including the manor of Brithdir) and elsewhere in Montgomeryshire, and to a lesser extent in Denbighshire, Merioneth, Shropshire, Cheshire and Lancashire.

2017: Four scrapbooks (one disbound), c.1857-c.1952, eleven letter books, 1874-1906, three photograph albums, bundles of letters, 1880-1900, and three game books, 1900-1950. Bundles of deeds, letters and other papers related to the purchase and sale of properties, mainly in p. Llanfyllin, c.1851-c.1954. Manuscript 'History and topography of the hundred of Llanfyllin', by "Mechain", 1893, notes for a history of Llanfyllin, c.1893-1916, and a typescript 'History of the parish of Llanfyllin from 1862 to 1913', by J. Marshall Dugdale, c.1916.

Deeds and documents relating to the Llwyndyrys estate and other properties in the parish of Llandygwydd, Cardiganshire, 1730-1923, including the Ddôl estate.

Manuscripts and records of the Llwyngwair estate in Pembrokeshire and Carmarthenshire, and of associated families, particularly the Bevans of Laugharne, including account books and rentals, 1689-1957; deeds, 1549-1884; manuscript maps of parts of the estate, 18-20 cent.; records of the Llwyngwair Estates Company, 1937-1953; accounts with traders in London, Cardigan, and of the Crymmych Arms, 1869-1903, accounts of servants' wages, 1914-1931; newspaper cuttings of family and local interest, 1866-1912; game and fishing registers, 1852-1940; and an album of photographs.

The so-called Llwynwormwood MS, containing legal precedents, many of them of Carmarthenshire and Pembrokeshire interest, medical and culinary recipes, etc.

Llyfr Aur Eisteddfod Genedlaethol Pwllheli, a luniwyd gan Gruffydd Parry (dyblygiad). Byrddau. Rhoddwyd gan Bwyllgor Eisteddfod Genedlaethol Pwllheli, trwy law Gruffudd Parry, Medi 1955.

A tune and song book in the hand of David Thomas, miller, of Pentrefoelas, co. Denbigh, previously of Felin Pandy, Penmachno, co. Caernarvon. Bound in at the beginning of the volume is Rheolau Cymdeithas Gantorawl Cerrig y-druidion . . . a sefydlwyd Chwefror 28, 1838.

An account book of Horeb Calvinistic Methodist Chapel, Horeb, Rhostryfan, 1850-66, in the autographs of W. Hughes, Coed-y-brain, and D. Williams, Tan'rallt.

Llyfr casgliad misol Capel M. C. Bethel, Tanygrisiau.(Gynt Borth-y-gest MS 38.) Byrddau. Prynwyd o lyfrgell Mr R. E. Jones, Borth-y-gest, 1959-1961.

Llyfr Casgliad y Weinidogaeth (Cylchdaith Ystumtuen), Eglwys Salem, Mynydd Bach, 1938-56. Tu mewn i'r clawr blaen ceir enw a chyfeiriad David Mason, Glanfedw, Pontarfynach, hen dad-cu Erwyd Howells.

Llyfr casgliad yn ymwneud â thân yn Llwynrheolfach. (Gynt Oakford MS 91.) Gweler hefyd NLW MSS 14036-14060. Papur. Rhoddwyd gan Mr S. Jones, Oakford, Llanarth, Ionawr 1942.

A manuscript book of hymn-tunes and anthems owned by John Lewis, Pont Twelly Stores, Llandysul, Cardiganshire, 1869. The titles include 'O na bawn i fel Efe'; 'Llawen Floeddiwch'; 'Caned Preswylwyr y Graig'; 'Dyrchaf fy llygaid'' 'Mola di'r Arglwydd o Seion'; 'Myned i Fynu'; 'Beth wyliedydd am y nos?'; 'Y Gwlithyn'; and 'Y fordaith'.

A manuscript music book belonging to Owen Jones (Owen y Cantwr), Penycae, Wrexham.