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The collection comprises: deeds and documents, 1617-1848, relating to properties in the Manor of Usk, Monmouthshire and Breconshire; and deeds and documents, 1586-1785, relating to properties in the county of Glamorgan.

Deeds relating to Cardigan, and St Dogmaels, Pembrokeshire, 1537-1804, predominantly of the property of the Weilshe family, 1563-1676, and the Davies family, 1676-1804; and deeds relating to Swansea, Glamorgan, 1821-1895.

Eleven letters, 1991-2002, from Kyffin Williams, Llanfairpwllgwyngyll, Anglesey, to his friends and near neighbours the broadcaster Ian Skidmore and his wife, the writer Celia Lucas, mainly offering thanks or congratulations, with most containing pen and ink self-portrait cartoons.
The correspondence includes four letters addressed to Celia Lucas (ff. 2-4, 10, the first two in French), three to Ian Skidmore (ff. 1, 9, 11) and two addressed to both (ff. 6, 8); together with a poem concerning the writer and critic A. A. Gill (f. 7) and a limerick addressed to Skidmore (f. 11). The cartoons portray Kyffin in a dunce cap (f. 1), as a Frenchman (f. 2 verso), as a 'naughty little boy' (f. 4 verso), celebrating (f. 5), with an ear trumpet (f. 6 verso), as [?'a fox-hunting man'] (f. 8), dancing with Ian Skidmore (f. 9) and waving a handkerchief (f. 10). There are also cartoons of A. A. Gill being grilled by Old Nick (f. 7) and Ian Skidmore waving a flag (f. 11).

Papers of Sir Kyffin Williams, 1716-[2008], including correspondence, 1923-2006; diaries and journals, 1939-2006; catalogues of, and papers regarding, solo and group exhibitions, 1950-2006; drafts of books and articles by Kyffin Williams, [?1965]-[?2004]; works about him, 1953-[2008]; financial papers, 1939-2005; personal papers, 1931-2006; together with papers relating to various family members, 1716-2006, and papers accumulated by the artist, 1796-2007.

Kyffin Williams photographs include personal and professional, family, Welsh views, artworks and views abroad, most notably Patagonia.

Research, 1993-1994, compiled by Dr Glyn Rhys concerning the Ceredigion ancestry of Sir Kyffin Williams.

A copy of the donor's genealogical research.

Papers of the Knowling Lentier family, [c. 1920s]-[c. 1930], including address book; correspondence, 1923; slides; and photographs, including one of David Lloyd George, and two of his daughter Lady Olwen Carey-Evans.

Instructions for knitting and crocheting lace.

Papers of and collected by Kitty Idwal Jones, 1797-1982, including, research papers of Professor Idwal Jones (1901-1965), relating to Rev. Thomas Jones (1756-1820), comprising printed works, obituaries, transcripts and typescripts of letters, 1797-1820, [1937x1984]; papers and correspondence accumulated by Kitty Idwal Jones relating to the history of Stonehenge, 1909-1959; papers relating to and created by Morfydd Llwyn Owen, [1894x1982], including letters from Morfydd Llwyn Owen; papers relating to voluntary work, 1916-1944; together with some papers relating to her time spent as a missionary in India, 1924-1979 and to a visit to America, 1928-1932; correspondence, 1912-1981; and miscellanea, [1905x1958].

A collection of manuscripts containing pedigrees and genealogical material relating mainly to North Wales; extracts, etc. from Anglesey, Caernarvonshire, Denbighshire and Flintshire deeds; accounts, [17 cent.]-[19 cent.], of the Ty Fry estate, Anglesey; transcripts by Angharad Llwyd; material relating to David Hughes, founder of the free grammar school, Beaumaris; extracts from Anglesey public records and other notes and transcripts relating to Anglesey; a calendar relating to the Courts of Great Sessions for Flintshire and Denbighshire, 1668-1696; correspondence collected by John Lloyd, Caerwys (1733-1793); Caerwys churchwardens' accounts, 1662-1669, 1680-1690, 1697-1698; material relating to Abergele; miscellaneous transcripts, extracts and translations; etc.

Deeds, 1313-[1825], from the collection of Angharad Llwyd (1779-1866), antiquary, including deeds relating to the Salusbury family of Lleweni, 1313-1727, and one to the Myddelton family of of Chirk, [c.1640].

A letter dated 26 August 1665, signed by King Charles II (1630-1685) and sent, per the Earl of Carlingford [d. 1677], from Salisbury, whither the English Court had removed owing to the plague, to 'Mon Cousin, L'Euesque de Munster', i.e. Christopher Bernard von Ghalen, prince-bishop of Munster, Westphalia, ally of England in the Anglo-Dutch war.

A copy of Richard Blackmore: King Arthur. An Heroick Poem ... (London, 1697), with manuscript notes explaining the numerous names (some of which are veiled) and classical references in the text.

Letter-book of Thomas Bowen of Pen-bre, co. Carmarthen, superintendent of the Kidwelly and Llanelly Canal and Railway Co., comprising an inventory of the company's records, 1831 (ff. 1-4), copy and draft letters, 1838-1840 (ff. 5-136 verso), a humorous poem on the failures of an anonymous colliery proprietor (ff. 151-5) and an arithmetical problem in Welsh, English and Latin (ff. 155 verso-6).

Minute book, November 1898 - February 1906, of the Kerry [co. Montgomery], Mutual Improvement Association. Inset are letters from [Doctor] F[rederick] Wilson, Newtown, to Mr. [Alexander] Anderson [secretary of the Association ], [19]05 (a promise to give a magic-lantern lecture on 'Infection'), and from John Naylor, Leighton Hall, Welshpool, to [ ], [19]05 (accepting the presidency of the Association for the ensuing year).

A register, 1898-1903, of members of the Kerry [co. Montgomery], Mutual Improvement Association, with a record of their attendances at meetings. At the reverse end of the volume are incomplete lists of officers of the Association during the same period.