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A copy of Alun R. Jones's typescript work 'Cymreictod y Creunant. Ffactorau sydd wedi dylanwadu ar hynt y Gymraeg yn y Creunant', 1993, relating to the decline of the Welsh language in the village of Creunant, co Glamorgan.

'Cofnodion Cymdeithas Cymreigyddion Cyfeiliog', being the minute book of the society, 1899-1917.

Printers' files and related papers relating to divisional Labour Party general and local government election pamphlets, posters and addresses, 1950-1986; Cardiff May Day Rally, 1964-1965; Cardiff ward branches, 1961-1986; the Welsh Centre for International Affairs, 1973-1986; and Brynlliw Lodge and the National Union of Mineworkers (South Wales Area), 1953-1984.

Minutes of committees and meetings of Cymdeithas Cymrodorion Aberdâr, 1907-1922.

Photocopied press cuttings relating to the activities, 1982-2007, of Cymru Cuba and celebrations held to mark the 25th anniversary of solidarity between Wales and Cuba.

Administrative records, publications and campaigning material of the socialist Welsh nationalist organisation Cymru Goch; containing minutes of committees, conference documents, correspondence, policy and discussion papers; newsletters and monograph publications.

The editor's own set of Cymru (O. M. Edwards), Vols. 1-44, 1891-1913 containing manuscript notes, some original manuscripts of contributions and letters by correspondents.

A volume of manuscript notes with insets (mostly newspaper cuttings, a few letters, etc.) compiled by Ionawryn Williams [of Manchester and Bethesda], and consisting mainly of biographical data relating to Welshmen who had resided in or been connected with the city of Manchester or the neighbourhood in the nineteenth century, including such figures as Robert Jones Derfel, the Reverend William James , and John Jones ('Poet Jones'), etc. A few of the entries refer to the compiler's previously published work on Manchester Welshmen entitled [Geirlyfr bywgraffiadol yn cynhwys byr-hanes y Cymry mwyaf adnabyddus fuont yn preswylio yn Manceinion, Salford, 1896]. The volume also contains an account of attempts to form a Welsh [literary] society in Manchester in 1835. Amongst the insets is a long autograph letter from R[ichard] J[ones] Berwyn, Trerauson Chwbut [sic] [Patagonia], to Ionawryn Williams, [18]97 ( a reply to a request for information concerning Thomas Penant Evans ('Twmi Dimol'), who had been one of the emigrants who had sailed to Patagonia in the Mimosa in 1865), and a short holograph note from the same writer to [Ionawryn Williams], undated (giving a few autobiographical details).

Papers, [1600x1924], mostly of or relating to Robert Ellis (Cynddelw), with some in the hand of Dr Robert Ellis, his son. The material includes a draft autobiography of Robert Ellis; an introduction written for a collection of Ellis's work under the proposed title Mwyar Berwyn; a draft of part of the first chapter of a biography of John Williams, Baptist minister (Llangollen, 1871); notes for Esboniad ar y Testament Newydd Cyfrol III (Llangollenn, 1878); poetry; diaries, 1840-1866; correspondence, 1833-1875; sermons; lectures; essays; adjudications at eisteddfodau, [1860x1875]; and miscellaneous notes, transcripts and extracts. The collection also includes letters, 1835-1856, of John Williams, Baptist minister; a rental, 1725-1726, of the estate of Watkin Williams Wynn; commonplace books of John Davies, Pentrefoelas, Griffith Williams (Gutyn Peris) and others, together with further collections of miscellany in seventeenth and eighteenth century hands; and autograph sermons by Christmas Evans.

Llungopïau o gynhyrchion cwrdd cystadleuol a gynhaliwyd yn eglwys y Bedyddwyr, Bethel, Mynachlog-ddu, sir Benfro, 30 Ionawr 1885, sef 'Hanes Eglwys Bethel...' gan 'Bachgennyn' (Benjamin Jenkins, Tycanol, Mynachlog-ddu), 'Traethawd ar Blwif Mynachlogddu' gan 'Standly', a beirniadaethau gan y Parch. Henry Price, gweinidog eglwys y Bedyddwyr, Rhydwilym.

Cynllaith Owen court leet records, 1736-1835, including court files, 1736-1758, presentments, 1815-1835, and estreats of fines, 1824-1835. There is also a single item from the manor of Nantymeichied, 1750, and four miscellaneous papers, 1816-1831.

'Cynllun Sabbathol Pregethwyr y Trefnyddion Wesleyaidd', Cylchdaith Aberteifi, Tachwedd 1842 - Chwefror 1843.

A holograph essay on 'Cynydd a gwelliant Llanbedr [Pont Steffan] yn ystod y 15 mlynedd diweddaf (1863-1878)' [the development and improvement of Lampeter, co. Cardigan, during the period 1863-1878] by 'Ap Tulas' [Dan Jenkins, Pentrefelin, Nantcwnlle, co. Cardigan]. The essay was awarded the first prize in an unspecified competition.

Original manuscripts of poems submitted for competition at 'Arwest Farddonol Glan Geirionydd' and other 'eisteddfodau', 1880-1894; and notes of an address and adjudications by W[illiam] J[ohn] Roberts ['Gwilym Cowlyd'] at Eisteddfod Meirion, Dolgellau, 1881.

A collecting book containing a printed statement of 'The Educational Difficulty at Cynwyd', Merioneth, 1887, and a list of subscribers for the establishment of a board school there.

Baptismal register, 1837-1900 (watermark 1836) of Cyssegr Congregational Church, Rhewl, Mostyn, Flintshire. The volume also contains transcripts of baptismal entries, 1832-1837, taken from an earlier register which was subsequently deposited with the Registrar General, and is now held in The National Archives. Most of the entries in this volume are in the hands of the Reverends Hugh Pugh and E. Pan Jones, successive ministers of Cyssegr Congregational Church.
Also included is a list of marriages solemnised at Cyssegr, 1837-1868 (ff. 73 verso-75 verso); an extract from the chapel deed (f. ii); copies of baptismal entries, 1824-1833, for the children of the Reverend William Rees ('Gwilym Hiraethog'), Hugh Pugh's predecessor as minister of Cyssegr Congregational Church (f. ii verso); and, loose at the beginning of the volume, a newspaper cutting, [1949], relating to the donation of the manuscript to the National Library of Wales.

Four duets for tenor and baritone to the words 'Y ddau Awenydd', submitted to the New York Eisteddfod of 22 February 1886 by 'Jakie' (J. W. Parson Price), 'Prydeiniwr' (W. Ellis, 'Alaw Cynan', Carneddi), 'Apontini' and 'Bertini', with the adjudicator's remarks.

A manuscript containing a 19th century transcript of a cywydd by David Vaughan, 1643, with an English translation under the title 'An Address to Sir John Pryce of Newtown, Bart, exciting him to Arms in support of Charles 1st ...'