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Account book, 1887-1916, of Thomas Jones, Pant-teg, Bronnant, co. Cardigan, weaver, with a few later memoranda, 1921-1924, mostly concerning machinery, by his son E. D. Jones. Note on 'Patrwn Carthen Felinfach' inside back cover.

Account book, mainly in Welsh, 1867-1907, of Thomas Jones (d. 1897), Brynmeheryn, Ystradmeurig, co. Cardigan, containing customers' accounts for weaving, sometimes with details of patterns; also included are a few veterinary recipes. Later entries are in the hand of Evan W. Jones, possibly the son of Thomas Jones.

Deeds and documents relating to properties mainly in Montgomeryshire, 1615-1910.

A typescript copy of an unpublished work by Richard Anthony entitled 'Water over Wales's Valleys', 1985.

Deeds, wills and other documents relating to Monmouthshire, 1568-1825.

Particulars, in the autograph of Walter Davies (Gwallter Mechain) (1761-1849), of wages paid to agricultural workers in Wales c. 1800.

Correspondence and other papers used in preparation towards the Wales Assembly of Women's report for the United Nations Fourth World Conference on the status of women, Beijing, 1995.

A notebook containing notes on the history and practice of the Courts of Great Sessions in Wales accumulated by W. Llewelyn Williams, K.C., M.P. (1867-1922) (see Y Cymmrodor, XVI, pp. 1-87). Many of the extracts are taken from the Llwynwormwood MS, i.e. NLW MS 4492D.

Deeds and documents relating to Cardiganshire, 1590-1751; and Montgomeryshire, 1517-1770; deeds and documents relating to the Hughes family of Gogarth, 1669-1910; and miscellaneous items, 1692-1825.

Deeds relating to properties at Deep Dean, Walford, Herefordshire, 1799-1816, and in Merthyr Tydfil, Glamorgan, 1788-1859.

Deeds relating to the parishes of Llanbadarn Fawr, 1548-1597, and Llangynfelyn, 1841-1848, Cardiganshire.

Two volumes containing manuscript music, 1809-1828, one inscribed within by 'Mary Madocks, alias Williams, Vron-Iw, October 1809', and two volumes of printed music, one of which belonged to Mrs Henry Laird, inscribed within by 'Jessie Laird, 1879', and bearing the initials 'J.L.', and the other bearing the bookplate of Mrs Mevekson-Sandbach. One manuscript copy and a printed copy has 'Mrs Williams, 1822' written on their covers.

Records of the Vale of Neath Brewery, 1844-1913, including ledgers, 1894-1897; pay books, 1882-1912; purchase abstract books, 1896-1908; beer sales books, 1896-1913; spirit sales books, 1897-1912; and printed books, 1863-1913.

Records of Vale of Glamorgan Liberal Association and Barry Constituency Liberal Association, comprising minutes of Annual General Meetings, 1974-1982; Executive Committee minutes, 1975-1987, papers relating to the Welsh Liberal Party, 1982-1987; Barry Town Liberal Association accounts, 1975-1984; correspondence concerning Prospective Parliamentary Candidate, 1981-1982 and with Vale of Glamorgan SDP, 1981-1985; notes on environment and planning in South Glamorgan, 1981-1982; general correspondence and papers, 1982-1987, including the proposed amalgamation with the SDP, 1987; election literature, 1983-1987; and papers relating to Sully and Wenvoe branches, 1983-1986.

Notes for a guided tour of the commote Uwch Aled, Denbighshire written by Robin Gwyndaf, 2011.

Account book, 1898-1918, of John Thomas, Rhoshelyg, Dinas Cross, co. Pembroke, undertaker and carpenter, with a few entries for 1880 and later additions, 1932-1942.

Minute-book of the Union of Welsh Teachers from its formation in 1926 up to 1938.

Holograph manuscripts of three tenor solos composed in 1930 by Thomas Hubert J. Rees - 'Y Gwylanod', 'Y Seren Unig', and 'Y Cwmwl', words by Sir John Morris-Jones.

A typescript copy of Alun Trevor's reminiscences of his childhood in north east Wales during the 1920s, and his life and career afterwards, entitled The songbird is singing (published by Parthian Books, 2009).

Papers relating to the Society for the Development of Tregaron and District (Cymdeithas Datblygu Tregaron a'r Cylch) comprising a minute book and draft minutes, 1967-1982; correspondence, 1967-1982; financial papers, 1967-1979; papers, 1969, relating to a survey by the Mid-Wales Industrial Development Association into the availability of labour in the Tregaron Rural District; and miscellaneous reports and printed booklets.